What was thought of as noise, points to new type of ultrafast magnetic switching

No magnetic effect, but fluctuations

This approach has now proved successful when investigating antiferromagnets. Antiferromagnets are magnetic materials in which the magnetizations of several sub-lattices cancel out each other. Nevertheless, antiferromagnetic insulators are considered promising for energy-efficient components in the field of information technology. As they have hardly any magnetic fields on the outside, they are very difficult to characterize physically. Yet, antiferromagnets are surrounded by magnetic fluctuations, which can tell us a lot about this weakly magnetic material.

In this spirit, the groups of the two materials scientists Ulrich Nowak and Sebastian Gönnenwein analysed the fluctuations of antiferromagnetic materials in the context of the CRC. The decisive factor in their theoretical as well as experimental study, recently published in the journal Nature Communications, was the specific frequency range. "We measure very fast fluctuations and have developed a method with which fluctuations can still be detected on the ultrashort time scale of femtoseconds," says experimental physicist Sebastian Gönnenwein. A femtosecond is one millionth of a billionth of a second.

New experimental approach for ultrafast time scales

On slower time scales, one could use electronics that are fast enough to measure these fluctuations. On ultrafast time scales, this no longer works, which is why a new experimental approach had to be developed. It is based on an idea from the research group of Alfred Leitenstorfer, who is also a member of the Collaborative Research Centre. Employing laser technology, the researchers use pulse sequences or pulse pairs in order to obtain information about fluctuations. Initially, this measurement approach was developed to investigate quantum fluctuations, and has now been extended to fluctuations in magnetic systems. Takayuki Kurihara from the University of Tokyo played a key role in this development as the third cooperation partner. He was a member of the Leitenstorfer research group and the Zukunftskolleg at the University of Konstanz from 2018 to 2020.

Detection of fluctuations using ultrashort light pulses

In the experiment, two ultrashort light pulses are transmitted through the magnet with a time delay, testing the magnetic properties during the transit time of each pulse, respectively. The light pulses are then checked for similarity using sophisticated electronics. The first pulse serves as a reference, the second contains information about how much the antiferromagnet has changed in the time between the first and second pulse. Different measurement results at the two points of time confirm the fluctuations. Ulrich Nowak's research group also modelled the experiment in elaborate computer simulations in order to better understand its results.

One unexpected result was the discovery of what is known as telegraph noise on ultrashort time scales. This means that there is not only unsorted noise, but also fluctuations in which the system switches back and forth between two well-defined states.Such fast, purely random switching has never been observed before and could be interesting for applications such as random number generators. In any case, the new methodological possibilities for analyzing fluctuations on ultrashort time scales offer great potential for further discoveries in the field of functional materials.